TY - JOUR
T1 - Biomass burning and fungal spores as sources of fine aerosols in Yangtze River Delta, China – Using multiple organic tracers to understand variability, correlations and origins
AU - Xu, Jingsha
AU - Jia, Chunrong
AU - He, Jun
AU - Xu, Honghui
AU - Tang, Yu Ting
AU - Ji, Dongsheng
AU - Yu, Huan
AU - Xiao, Hang
AU - Wang, Chengjun
N1 - Publisher Copyright:
© 2019 Elsevier Ltd
PY - 2019/8
Y1 - 2019/8
N2 - Research is restricted regarding impacts of biomass burning (BB)on fine aerosol (PM2.5), due mainly to lack of specific BB tracers. This study aims to characterize the variability, distributions, and contributions of BB and fungal spores as sources of PM2.5 using a multiple organic tracer approach. PM2.5 samples were collected at four representative sites in Yangtze River Delta (YRD), China every 6 days for one year. In the laboratory, samples were analyzed for three anhydrides (levoglucosan, mannosan, and galactosan), two sugar alcohols (arabitol and mannitol), water-soluble inorganic ions, and elemental/organic carbon (EC/OC). Levoglucosan was the most abundant BB tracer (mean concentration = 81 ng/m3), and fungal spore tracers arabitol and mannitol had similar abundances (5.6 and 5.7 ng/m3, respectively). Anhydrides and sugar alcohols had high within-group correlations, indicating their respective common sources. Concentrations of tracers displayed large temporal variations but small spatial variations, suggesting strong seasonality in BB and fungal spore sources. BB sources were burning of grass, pine needles, hardwood and crop straw, which were originated from transboundary/cross-region transport and local fire spots. PCA analyses revealed that the common sources of fine aerosols in YRD were secondary inorganic aerosols, soil dust, BB and fungal spores.
AB - Research is restricted regarding impacts of biomass burning (BB)on fine aerosol (PM2.5), due mainly to lack of specific BB tracers. This study aims to characterize the variability, distributions, and contributions of BB and fungal spores as sources of PM2.5 using a multiple organic tracer approach. PM2.5 samples were collected at four representative sites in Yangtze River Delta (YRD), China every 6 days for one year. In the laboratory, samples were analyzed for three anhydrides (levoglucosan, mannosan, and galactosan), two sugar alcohols (arabitol and mannitol), water-soluble inorganic ions, and elemental/organic carbon (EC/OC). Levoglucosan was the most abundant BB tracer (mean concentration = 81 ng/m3), and fungal spore tracers arabitol and mannitol had similar abundances (5.6 and 5.7 ng/m3, respectively). Anhydrides and sugar alcohols had high within-group correlations, indicating their respective common sources. Concentrations of tracers displayed large temporal variations but small spatial variations, suggesting strong seasonality in BB and fungal spore sources. BB sources were burning of grass, pine needles, hardwood and crop straw, which were originated from transboundary/cross-region transport and local fire spots. PCA analyses revealed that the common sources of fine aerosols in YRD were secondary inorganic aerosols, soil dust, BB and fungal spores.
KW - Biomass burning
KW - Fungal spore
KW - Source identification
KW - Spatial variation
KW - Temporal variation
UR - http://www.scopus.com/inward/record.url?scp=85065476457&partnerID=8YFLogxK
U2 - 10.1016/j.envpol.2019.04.090
DO - 10.1016/j.envpol.2019.04.090
M3 - Article
C2 - 31078087
AN - SCOPUS:85065476457
SN - 0269-7491
VL - 251
SP - 155
EP - 165
JO - Environmental Pollution
JF - Environmental Pollution
ER -
